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JNC TJ8400 2000-017, 74 Pages, 2000/02
JNC-TJ8400-2000-017.pdf:1.71MB
The report concerns the improvement of the method measuring thermal conductivity of buffer materials using a thermistor probe and the measurement of thermal conductivity of compacted bentonites and mixtures of bentonite and silica sand using the proposed method measuring thermophysical properties. The method measuring thermal conductivity is improved in accuracy and the apparatus is improved so as to measure easily with more short time. The calculated values of the conventional correlations predicting thermal conductivity of bentonite and mixture were compared with the exising and present data of thermal conductivity of bentonites and mixtures. The correlation proposed by Sakashita and Kumada can predict the best fitted values with the data of the bentonites and Fricke and Bruggeman correlations are fitted with the data for the mixtures with practical accuracy.
Chijimatsu, Masakazu*; Fujita, Tomoo; Sugita, Yutaka; Taniguchi, Wataru
JNC TN8400 2000-008, 339 Pages, 2000/01
JNC-TN8400-2000-008.pdf:30.96MB
Geological disposal of high-level radioactive waste (HLW) in Japan is based on a multibarrier system composed of engineered and natural barriers. The engineered barriers are composed of vitrified waste confined within a canister, overpack and buffer material. Highly compacted bentonite clay is considered one of the most promising candidate buffer material mainly because of its low hydraulic conductivity and high adsorption capacity of radionuclides. In a repository for HLW, complex thermal, hydraulic and mechanical (T-H-M) phenomena will take place, involving the interactive processes between radioactive decay heat from the vitrified waste, infiltration of ground water and stress generation due to the earth pressure, the thermal loading and the swelling pressure of the buffer material. In order to evaluate the performance of the buffer material, the coupled T-H-M behaviors within the compacted bentonite have to be modelled. Before establishing a fully coupled T-H-M model, the mechanism of each single Phenomenon or partially coupled phenomena should be identified. Furthermore, in order to evaluate the coupled T-H-M phenomena, the analysis model was developed physically and numerically and the adequacy and the applicability was tested though the engineered scale laboratory test and in-situ test. In this report, the investigative results for the development of coupled T-H-M model were described. This report consists of eight chapters. In Chapter l, the necessity of coupled T-H-M model in the geological disposal project of the high-level radioactive waste was described. In Chapter 2, the laboratory test results of the rock sample and the buffer material for the coupled T-H-M analysis were shown. The rock samples were obtained from the in-situ experimental site at Kamaishi mine. As the buffer material, bentonite clay (Kunigel V1 and Kunigel OT-9607) and bentonite-sand mixture were used. In Chapter 3, in-situ tests to obtain the rock property were shown. As ...
Tanai, Kenji; Sato, Haruo; *; *
JNC TN8400 99-045, 108 Pages, 1999/11
In the anaerobic environment in the deep underground water, carbon-steel overpack corrodes and generates molecular hydrogen. It is conceivable that this hydrogen either dissolves into the porewater of the buffer and migrates through the buffer. If the rate of aqueous diffusion of hydlogen is too low compared to the rate of hydrogen generation, the concentration of hydrogen at the overpack surface will increase until a solubility limit is attained and a free hydrogen gas phase forms. It is possible that the pressure in this accumulating gas phase will increase, affecting the stability of the buffer or the surrounding rock mass. There is also a concern of possible effects on nuclide migration, as it is also conceivable that the flow of gas could push out radionuclide-bearing porewater in the buffer when it floes through the buffer. As such, experimental and analytical study must be carried out on such phenomenon to evaluate such potential phenomena. (1)Diffusion experiment of dissolved hydrogen. According to the test result concerning the effective diffusion coefficient of the dissolved hydrogen in buffer material, the effective diffusion coefficient of reference buffer material (70wt% bentonite + 30wt% sand mixture, dry density 1.6Mg m
) ranges from 10
m
s
to 10
ms. The value of the effective diffusion coefficient measured for a dry density of 1.8 Mg m is slightly smaller than the value in that for a dry density 1.6 Mg m. And the effective diffusion coefficient at 60
C tends to have slightly larger value than that at 25C. Test results from the foreign countries show the diffusion coefficient in the range between 10
ms to 10
ms. Basically, these test results reported here are in the same range as these other results. (2)Gas permeability. Studies of the gas permeabinty of buffer material have been carried out by Pusch et al., Volckaert ...
Takachi, Kazuhiko; Suzuki, Hideaki*
JNC TN8400 99-041, 76 Pages, 1999/11
The buffer material is expected to maintain its low water permeability, self-sealing properties, radionuclides adsorption and retardation properties, thermal conductivity, chemical buffering properties, overpack supporting properties, stress buffering properties, etc. over a long period of time. Natural clay is mentioned as a material that can relatively satisfy above. Among the kinds of natural clay, bentonite when compacted is superior because (1)it has exceptionally low water permeability and properties to control the movement of water in buffer, (2)it fills void spaces in the buffer and fractures in the host rock as it swells upon water uptake, (3)it has the ability to exchange cations and to adsorb cationic radioelements. In order to confirm these functions for the purpose of safety assessment, it is necessary to evaluate buffer properties through laboratory tests and engineering-scale tests, and to make assessments based on the ranges in the data obtained. This report describes the procedures, test conditions, results and examinations on the buffer material of unconfined compression tests, one-dimensional consolidation tests, consolidated-undrained triaxial compression tests and consolidated-undrained triaxial creep tests that aim at getting hold of static mechanical properties. We can get hold of the relationship between the dry density and tensile stress etc. by Brazillian tests, between the dry density and unconfined compressive strength etc. by unconfined compression tests, between the consolidation stress and void ratio etc. by one-dimensional consolidation tests, the stress pass of each effective confining pressure etc. by consolidated-undrained triaxial compression tests and the axial strain rate with time of each axial stress etc. by consolidated-undrained triaxial creep tests.
Sugita, Yutaka; Fujita, Tomoo; Tanai, Kenji; Hasegawa, Hiroshi; Furuichi, Mitsuaki*; Okutsu, Kazuo*; Miura, K.*
JNC TN8400 99-039, 58 Pages, 1999/11
Regarding disposal techniques of high-level radioactive waste (HLW), the HLW is vitrified and then stored for cooling for a period of 30 to 50 years. After cooling, the HLW is isolated in the deep underground. The concept of geological disposal is based on the requirement to enclose the HLW in the deep underground for the long-term durability of the human's environmental safety. Backfilling of a repository is a unique activity on the geological disposal. If underground tunnels excavated to construct the repository are left, they may have significant influences on the barrier performance of an entire repository, such as: the mechanical stability of a tunnel may be damaged by rock stresses and a tunnel may provide a fast pathway for ground water flow. Therefore, the underground facilities are expected to be backfilled with a backfilling material after emplacement of the HLW and a buffer material. The material for the backfilling of the underground facilities is backfilling material. In this report, bentonite-aggregate mixture is considered, as one of the candidate materials for the backfilling material. Aggregate imitates the muck that is generated during construction phase of the underground facilities. The combination of backfilling, plugging and grouting is considered in some underground situations. Plug is composed of concrete material or clay-based one. Grouting material is concrete material or clay-based one, too. In this report, the concept of the backfilling, mechanical and hydrological characteristics of the bentonite-aggregate mixture, the function, work methods and a schedule of the backfilling materials, plugging and grouting are considered, and items of quality control for the bentonite-aggregate mixture, concrete material and grouting are listed.
Sato, Haruo
JNC TN8400 99-064, 22 Pages, 1999/10
Four kinds of diffusion experiments; (1)through-diffusion(T-D) experiments for compaction direction dependency, (2)in-diffusion(I-D) experiments for composition dependency of silica sand in bentonite, (3)I-D experiments for initial bentonite gain size dependency, and (4)I-D experiments for the restoration property of an artificial single fracture in compacted bentonite, were carried out using tritiated water which is a non-sorbing nuclide to evaluate the effect of pore structural factors for eompacted bentonite on diffudion. For(1), effective diffusivities (De) in Na-bentonites, Kunigel-V1 and Kunipia-F were measured for 1.0 and 1.5 Mg
m. For(2), apparent diffusivities (Da) in Kunigel-V1 were measured for 0.8, 1.4 and 1.8 Mgm with silica sand of 30 and 50 wt%. For(3), Da values for 0.8, 1.4 and 1.8 Mgm were measured for a granulated Na-bentonite, OT-9607 which grain-size distribution is in a rang between 0.1 and 5 mm. For (4), Da values in Kunigel-V1 which a single fracture was artificially reproduced and was immersed in distilled water for 7 or 28 days for the restoration of the fracture, were measured for 1.8 Mgm. Although De values in Kunigel-V1 were approximately the same for both compacted directions over the density, De values for perpendicular direction to compacted direction were higher than those for the same direction as compacted direction in Kunipia-F. For composition dependency of silica sand in bentonite, no significant effect of the mixure of silica sand in bentonite on Da was found. For initial bentonite grain size dependency, Da values obtained for OT-960 were approximately the same as those for Kunigel-V1 and no effect of initial grain size of bentonite on diffusion was found. For the restoration property of a single fracture in compacted bentonite, no restoration period dependency on Da was found. Based on this, it may be said that diffusion of nuclides in compacted bentonite, ...
Sato, Haruo
JNC TN8400 99-060, 12 Pages, 1999/10
Apparent diffusion coefficients(Da) of Cs(Cs
), Ni(Ni
) and Se(SeO
) in a Na-bentonite (Kunigel-V1) were measured for a dry density of 1.8 Mgm with silica sand of 30 wt% at room temperature by in-diffusion method to evaluate the effect of the mixture of silica sand on Da in bentonite. The experiments for Cs and Ni were carried out under aerobic condition, but those for Se which is redox sensitive were carried out in an Ar glove-box (O
concentration 
0.1 ppm). Consequently, no significant effect of silica sand mixture to the bentonite on Da values of Cs and Se was found, and the obtained Da values were approximately the same as those in the system without silica sand reported so far. On the other hand, Da values of Ni in bentonite with silica sand were 2 orders of magnitude lower than those in bentonite without silica sand obtained to date. The Da values of Ni reported so far were obtained using stable isotopic tracer and a tracer solution with fairly high Ni concentration compared with concentration used in this study was introduced. Additionally, it is known that distribution coefficient (Kd) of Ni on Na-montmorillonite which is the major constituent clay mineral of Kunigel-V1 decreases with increasing Ni concentration. Based on this, the abrupt decrease in Da values of Ni for bentonite with silica sand is considered to be due to the difference of sorption caused by the difference of Ni concentration in the porewater of bentonite.
Ueta, Shinzo*
PNC TJ1211 98-002, 46 Pages, 1998/02
None
Ueta, Shinzo*
PNC TJ1211 98-001, 824 Pages, 1998/02
None
Fukazawa, E.*; Tanaka, M.*; Yamamoto, H.*; Taira, K.*; Yamamoto, M.*; Okutsu, Kazuo*; Hane, Koji*; Aoyagi, Takayoshi*; Morikawa, Seiji*; Furuichi, Mitsuaki*
PNC TJ1100 98-006, 434 Pages, 1998/02
None
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PNC TJ1211 97-010, 23 Pages, 1997/03
None
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PNC TJ1211 97-009, 620 Pages, 1997/03
None
Hibiya, Keisuke*; *; Shiogama, Yukihiro*; Masumoto, Kazuhiko*; Fukazawa, E.*; Taira, K.*; Tanaka, Toshiyuki*; Kondo, Y.*; Yamamoto, M.*; Okutsu, Kazuo*; et al.
PNC TJ1100 97-004, 69 Pages, 1997/02
None